In-situ polymerization induced Mn2O3 sites as intrinsic carbon defects for capacitive organic dye removal

Xiaonan Li, Xinhua Huang, Zhirou Wang, Ruikun Zhao, Xiaofeng Cao, Yanchuan Guo

Research output: Contribution to journalArticlepeer-review

9 Scopus citations

Abstract

This paper aims to explanation on the effects of pseudo-capacitance on the capacitive performance of defective carbon-based materials. A series composite samples of Mn2O3 doped porous carbon were prepared with combining N induced intrinsic defects, we testified it as the electrode for flow capacitive Rhodamine B (RhB) removal performance. It is proved that the presence of Mn2O3 can indeed supply additional defects and pseudo-capacitance. Furthermore, the optimized Mn2O3@NCT-2 presented high quality capacity of 200F/g at 1 A/g in 1.0 M NaCl. Our results also displayed an extremely high RhB-adsorption capacity of 766.5 mg/g at an applied voltage of 1.2 V. These acquired new knowledge could advance expand a significant defect-engineering tactics to further improve the desalination nature of electrode materials.

Original languageBritish English
Article number120583
JournalSeparation and Purification Technology
Volume287
DOIs
StatePublished - 15 Apr 2022

Keywords

  • Active sites
  • Capacitive Deionization
  • Pseudo-capacitance
  • RhB removel
  • Seperation

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