High-performance perovskite single-junction and textured perovskite/silicon tandem solar cells via slot-die-coating

Anand S. Subbiah; Furkan H. Isikgor; Calvyn T. Howells; Michele De Bastiani; Jiang Liu; Erkan Aydin; Francesco Furlan; Thomas G. Allen; Fuzong Xu; Shynggys Zhumagali; Sjoerd Hoogland; Edward H. Sargent; Iain McCulloch; Stefaan De Wolf

doi:10.1021/acsenergylett.0c01297

High-performance perovskite single-junction and textured perovskite/silicon tandem solar cells via slot-die-coating

Anand S. Subbiah
, Furkan H. Isikgor
, Calvyn T. Howells
, Michele De Bastiani
, Jiang Liu
, Erkan Aydin
, Francesco Furlan
, Thomas G. Allen
, Fuzong Xu
, Shynggys Zhumagali
, Sjoerd Hoogland
, Edward H. Sargent
, Iain McCulloch
, Stefaan De Wolf

King Abdullah University of Science and Technology
MaRS Center
University of Toronto
University of Oxford

Research output: Contribution to journal › Article › peer-review

189 Scopus citations

Abstract

In this work, we report perovskite solar cells in the planar p-i-n configuration based on single-step, anti-solvent-free, low-temperature (70 °C) slot-die-coated methylammonium lead tri-iodide (MAPbI3). The devices are fabricated on hydrophobic poly(triarylamine) (PTAA) surfaces, using key strategies such as solvent engineering, enhanced ink-substrate dynamics, and surface passivation, enabling a power conversion efficiency (PCE) of 21.8%. We also adapted the technique to achieve the first slot-die-coated perovskite/silicon monolithic 2-terminal tandems, achieving a PCE of 23.8% utilizing a textured silicon bottom cell.

Original language	British English
Pages (from-to)	3034-3040
Number of pages	7
Journal	ACS Energy Letters
Volume	5
Issue number	9
DOIs	https://doi.org/10.1021/acsenergylett.0c01297
State	Published - 11 Sep 2020

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SDG 7 Affordable and Clean Energy

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Subbiah, A. S., Isikgor, F. H., Howells, C. T., De Bastiani, M., Liu, J., Aydin, E., Furlan, F., Allen, T. G., Xu, F., Zhumagali, S., Hoogland, S., Sargent, E. H., McCulloch, I., & De Wolf, S. (2020). High-performance perovskite single-junction and textured perovskite/silicon tandem solar cells via slot-die-coating. ACS Energy Letters, 5(9), 3034-3040. https://doi.org/10.1021/acsenergylett.0c01297

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title = "High-performance perovskite single-junction and textured perovskite/silicon tandem solar cells via slot-die-coating",

abstract = "In this work, we report perovskite solar cells in the planar p-i-n configuration based on single-step, anti-solvent-free, low-temperature (70 °C) slot-die-coated methylammonium lead tri-iodide (MAPbI3). The devices are fabricated on hydrophobic poly(triarylamine) (PTAA) surfaces, using key strategies such as solvent engineering, enhanced ink-substrate dynamics, and surface passivation, enabling a power conversion efficiency (PCE) of 21.8\%. We also adapted the technique to achieve the first slot-die-coated perovskite/silicon monolithic 2-terminal tandems, achieving a PCE of 23.8\% utilizing a textured silicon bottom cell.",

author = "Subbiah, \{Anand S.\} and Isikgor, \{Furkan H.\} and Howells, \{Calvyn T.\} and \{De Bastiani\}, Michele and Jiang Liu and Erkan Aydin and Francesco Furlan and Allen, \{Thomas G.\} and Fuzong Xu and Shynggys Zhumagali and Sjoerd Hoogland and Sargent, \{Edward H.\} and Iain McCulloch and \{De Wolf\}, Stefaan",

note = "Funding Information: The authors acknowledge the support of the King Abdullah University of Science and Technology (KAUST) Office of Sponsored Research (OSR) under Award KAUST OSR-CARF URF/1/3097, as well as funding support from QD Solar, Inc. The authors also thank the members of the KAUST Solar Center operations team for their valuable support. The authors also thank all the previous reports tabulated in Table S5 for the data points compiled in the TOC graphic. Publisher Copyright: Copyright {\textcopyright} 2020 American Chemical Society.",

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doi = "10.1021/acsenergylett.0c01297",

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Subbiah, AS, Isikgor, FH, Howells, CT, De Bastiani, M, Liu, J, Aydin, E, Furlan, F, Allen, TG, Xu, F, Zhumagali, S, Hoogland, S, Sargent, EH, McCulloch, I & De Wolf, S 2020, 'High-performance perovskite single-junction and textured perovskite/silicon tandem solar cells via slot-die-coating', ACS Energy Letters, vol. 5, no. 9, pp. 3034-3040. https://doi.org/10.1021/acsenergylett.0c01297

TY - JOUR

T1 - High-performance perovskite single-junction and textured perovskite/silicon tandem solar cells via slot-die-coating

AU - Subbiah, Anand S.

AU - Isikgor, Furkan H.

AU - Howells, Calvyn T.

AU - De Bastiani, Michele

AU - Liu, Jiang

AU - Aydin, Erkan

AU - Furlan, Francesco

AU - Allen, Thomas G.

AU - Xu, Fuzong

AU - Zhumagali, Shynggys

AU - Hoogland, Sjoerd

AU - Sargent, Edward H.

AU - McCulloch, Iain

AU - De Wolf, Stefaan

N1 - Funding Information: The authors acknowledge the support of the King Abdullah University of Science and Technology (KAUST) Office of Sponsored Research (OSR) under Award KAUST OSR-CARF URF/1/3097, as well as funding support from QD Solar, Inc. The authors also thank the members of the KAUST Solar Center operations team for their valuable support. The authors also thank all the previous reports tabulated in Table S5 for the data points compiled in the TOC graphic. Publisher Copyright: Copyright © 2020 American Chemical Society.

PY - 2020/9/11

Y1 - 2020/9/11

N2 - In this work, we report perovskite solar cells in the planar p-i-n configuration based on single-step, anti-solvent-free, low-temperature (70 °C) slot-die-coated methylammonium lead tri-iodide (MAPbI3). The devices are fabricated on hydrophobic poly(triarylamine) (PTAA) surfaces, using key strategies such as solvent engineering, enhanced ink-substrate dynamics, and surface passivation, enabling a power conversion efficiency (PCE) of 21.8%. We also adapted the technique to achieve the first slot-die-coated perovskite/silicon monolithic 2-terminal tandems, achieving a PCE of 23.8% utilizing a textured silicon bottom cell.

AB - In this work, we report perovskite solar cells in the planar p-i-n configuration based on single-step, anti-solvent-free, low-temperature (70 °C) slot-die-coated methylammonium lead tri-iodide (MAPbI3). The devices are fabricated on hydrophobic poly(triarylamine) (PTAA) surfaces, using key strategies such as solvent engineering, enhanced ink-substrate dynamics, and surface passivation, enabling a power conversion efficiency (PCE) of 21.8%. We also adapted the technique to achieve the first slot-die-coated perovskite/silicon monolithic 2-terminal tandems, achieving a PCE of 23.8% utilizing a textured silicon bottom cell.

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SP - 3034

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JO - ACS Energy Letters

JF - ACS Energy Letters

IS - 9

ER -

High-performance perovskite single-junction and textured perovskite/silicon tandem solar cells via slot-die-coating

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