A widely tunable difference-frequency-generation laser for high-resolution spectroscopy in the 667-865 cm-1range

Mohammad Khaled Shakfa, Marco Lamperti, Riccardo Gotti, Davide Gatti, Ali Elkhazraji, Khaiyom Hakimov, Marco Marangoni, Aamir Farooq

Research output: Chapter in Book/Report/Conference proceedingConference contributionpeer-review

7 Scopus citations

Abstract

Mid-infrared (MIR) laser sources are used in a number of applications such as remote sensing, air pollution monitoring, combustion diagnostics, and molecular spectroscopy. Here, we present our work on the development of a MIR laser source based on the difference frequency generation (DFG) process between an external-cavity quantum-cascade-laser tunable over 1750-1835 cm-1 (pump source) and a CO2 gas laser tunable over 921-1083 cm-1 (signal source). The DFG process was realized in a nonlinear, orientation-patterned GaAs crystal, and resulted in an idler spectral range between 667-865 cm-1 with a linewidth of ∼2.3 MHz and an output power of up to ∼31 μW. Exploiting the fine tunability of our DFG laser source, we performed high-resolution absorption measurements of ethylene (C2H4) and acetylene (C2H2).

Original languageBritish English
Title of host publicationNonlinear Frequency Generation and Conversion
Subtitle of host publicationMaterials and Devices XX
EditorsPeter G. Schunemann, Kenneth L. Schepler
PublisherSPIE
ISBN (Electronic)9781510641754
DOIs
StatePublished - 2021
EventNonlinear Frequency Generation and Conversion: Materials and Devices XX 2021 - Virtual, Online, United States
Duration: 6 Mar 202111 Mar 2021

Publication series

NameProceedings of SPIE - The International Society for Optical Engineering
Volume11670
ISSN (Print)0277-786X
ISSN (Electronic)1996-756X

Conference

ConferenceNonlinear Frequency Generation and Conversion: Materials and Devices XX 2021
Country/TerritoryUnited States
CityVirtual, Online
Period6/03/2111/03/21

Keywords

  • Difference frequency generation
  • High-resolution spectroscopy
  • Laser spectroscopy
  • Mid-infrared laser sources

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