A facile method to synthesis a mesoporous carbon supported methanol catalyst containing well dispersed Cu/ZnO

Huamei Duan, Yunxia Yang, Jim Patel, Deepa Dumbre, Suresh K. Bhargava, Nick Burke, Yuchun Zhai, Paul A. Webley

    Research output: Contribution to journalArticlepeer-review

    9 Scopus citations

    Abstract

    Alumina supported CuO/ZnO is the commercial catalyst for methanol synthesis from syngas. Though so far, this catalyst has been regarded as the dominant catalyst for methanol synthesis. The catalyst is still facing some fundamental challenges such as the dispersion of active center CuO/ZnO. Meanwhile, to prepare this catalyst, large amount of nitrate precursor was used and produced lots of environmentally harmful wastewater. In the current work, a bimodal carbon channel-confined CuO/ZnO supported on mesoporous carbon catalyst was synthesized by using a simple impregnation method followed by ammonia hydrolysis and pyrolysis. The results demonstrated that the method we developed was an effective way to control the dispersion of metal oxides particles.

    Original languageBritish English
    Pages (from-to)e232-e237
    JournalMaterials Research Bulletin
    Volume60
    DOIs
    StatePublished - Dec 2014

    Keywords

    • A. Structural materials
    • B. Microstructure
    • C. Transmission electron microscopy (TEM)
    • D. Catalytic properties

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